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synthesis, characterization, and photovoltaic properties of soluble tiopc derivatives合成、表征和可溶性tiopc光伏性质的衍生品.pdf

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Int. J. Mol. Sci. 2008, 9, 2745-2756; DOI: 10.3390/ijms9122745 OPEN ACCESS International Journal of Molecular Sciences ISSN 1422-0067 /journal/ijms/ Article Synthesis, Characterization, and Photovoltaic Properties of Soluble TiOPc Derivatives Young-Keun Kim 1, 2, Hyo-Jin Kang 1 , Young-Wook Jang 1, 2, Su-Bin Lee 1, Seung-Min Lee 1, Ki-Suck Jung 1, 3, Jin-Kook Lee 1,* and Mi-Ra Kim 1,* 1 Department of Polymer Science and Engineering, Pusan National University, Busan, 609-735, South Korea 2 Polycen Co., Ltd., Busan, 608-739, South Korea 3 Daehan Solvay Special Chemicals Co., Ltd., Ulsan, South Korea * Authors to whom correspondence should be addressed; E-Mails: leejk@pusan.ac.kr (J. L.), mrkim2@pusan.ac.kr (M. K.); Tel. +82-51-510-3045; Fax: +82-51-513-7720 Received: 20 November 2008; in revised form: 16 December 2008 / Accepted: 18 December 2008 / Published: 19 December 2008 Abstract: We have synthesized soluble TiOPc derivatives containing alkoxy groups for use as additives in dye-sensitized solar cells (DSSCs). The DSSC devices containing these TiOPc derivatives exhibited short-circuit current densities of 8.49~10.04 mA/cm2 and power conversion efficiencies of 2.73~3.62 % under AM 1.5 illumination and 100 mW/cm2 irradiation. Keywords: Titanyl phthalocyanine (TiOPc); Dye-sensitized solar cell; Polymer electrolyte. 1. Introduction Dye-sensitized solar cells (DSSCs) constructed using dye molecules, nanocrystalline metal

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